We show that the increasingly popular nonlinear optical technique of time-domain coherent anti-Stokes Raman scattering (CARS), which is often viewed from the dynamical perspective of the semiclassical time-dependent third-order polarization, can also be studied by means of the time-delayed version of the Yuratich equation, so popular in traditional frequency-domain CARS. The method proves successful in explaining experimental results that are otherwise treated by means of numerical methods only. © 2014 Optical Society of America.
Time-domain coherent anti-Stokes Raman scattering in terms of the time-delayed Yuratich equation
Marrocco, M
2014-01-01
Abstract
We show that the increasingly popular nonlinear optical technique of time-domain coherent anti-Stokes Raman scattering (CARS), which is often viewed from the dynamical perspective of the semiclassical time-dependent third-order polarization, can also be studied by means of the time-delayed version of the Yuratich equation, so popular in traditional frequency-domain CARS. The method proves successful in explaining experimental results that are otherwise treated by means of numerical methods only. © 2014 Optical Society of America.File in questo prodotto:
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